The Vigilante definitely didn't have ailerons, and I think your interpretation is essentially accurate, John. The spoiler deflection to apply bank would be proportional to the control input, and for that purpose would likely be limited to around 45 degrees of deflection (the 78 degrees figure would only be for lift-dump/airbrake application). The reverse-flow spoilers are mechanically linked to the conventional ones, and deploy whenever the normal spoilers are deployed.
This quote from Tailspin (see
here):
"There were two sets of spoiler, slot, and deflector on each wing (and no ailerons). The deflector was hinged on its aft side so it directed air into the slot; the spoiler was hinged on its forward side to open the slot for the deflected air to escape. One set raised that wing. The other set lowered it. The inboard set took up more of the span than the outboard set, presumably to equalize the rolling moment. If you look closely at the comparison pictures of the A3J and RA-5C above, you'll see two different roll-control configurations, one to roll left and one to roll right. I've added an illustration of the spoiler/slot/deflector.
Speed brake actuation opened all four sets of roll controls simultaneously. Roll control was then accomplished by partially closing the opposing sets, reducing speed brake effectiveness."
Edit: just noticed that you have the inboard and outboard spoilers acting in opposition. They don't; they act in unison. So both upper surface spoilers raise at the same time, though they may raise at different rates and angles. This system is a direct predecessor of what is used on almost all modern airliners, though modern fly-by-wire gives a far more nuanced and adjustable control algorithm.
More info
here. The small panel is an extract from the Technical Manual, which is about as authoritative as you're going to get!
Further Edit:
it would appear I'm wrong and you're right - the inner and outer spoilers do in fact act in opposition. The outer spoilers give the initial roll input and the inner spoilers increase the roll rate if demanded.